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論文

Nanometric fluctuations of sound velocity in alkali borate glasses and fragility of respective melts

小島 誠治*; Novikov, V. N.*; 古府 麻衣子; 山室 修*

Physica Status Solidi (B), 257(11), p.2000073_1 - 2000073_6, 2020/11

https://doi.org/10.1002/pssb.202000073
 被引用回数：3 パーセンタイル：19.68(Physics, Condensed Matter)

The network structure of borate glass is remarkably modified by the addition of alkali metals. The alkali metal dependences of the first sharp diffraction peak (FSDP) and the boson peak (BP) are investigated in alkali borate glasses by elastic and inelastic neutron scattering experiments. With an increase in ionic radius of alkali ions, both the width $$Delta Q$$ of FSDP and the BP energy decrease. The comparison of the characteristic length of medium-range order (MRO) predicted by the FSDP and the position of the BP allows us to find the mean-square fluctuations of the transverse sound velocity within series of alkali borate glasses. It is shown that the fragility of the respective alkali borate melts inversely correlates with the mean-square fluctuations of the transverse sound velocity in glassy state.

論文

Experimental realization of a passive Gigahertz frequency-division demultiplexer for magnonic logic networks

Heussner, F.*; Talmelli, G.*; Geilen, M.*; Heinz, B.*; Br$"a$cher, T.*; Meyer, T.*; Ciubotaru, F.*; Adelmann, C.*; 山本 慧; Serga, A. A.*; et al.

Physica Status Solidi; Rapid Research Letters, 14(4), p.1900695_1 - 1900695_6, 2020/04

https://doi.org/10.1002/pssr.201900695
 被引用回数：34 パーセンタイル：87.61(Materials Science, Multidisciplinary)

The emerging field of magnonics employs spin waves and their quanta, magnons, to implement wave-based computing on the micro- and nanoscales. Multi-frequency magnon networks would allow for parallel data processing within single logic elements whereas this is not the case with conventional transistor-based electric logic. However, a lack of experimental proven solutions to efficiently combine and separate magnons of different frequencies has impeded the intensive use of this concept. In this Letter, the experimental realization of a spin-wave demultiplexer enabling frequency-dependent separation of magnetic signals in the GHz range is demonstrated. The device is based on two-dimensional magnon transport in the form of spin-wave beams in unpatterned magnetic films. The intrinsic frequency-dependence of the beam direction is exploited to realize a passive functioning obviating an external control and additional power consumption. This approach paves the way to magnonic multiplexing circuits enabling simultaneous information transport and processing.

論文

Kinetics of silver photodiffusion into amorphous Ge$$_{20}$$S$$_{80}$$ films; Case of pre-reaction

坂口 佳史*; 花島 隆泰*; 青木 裕之; 朝岡 秀人; Simon, A.-A. A.*; Mitkova, M.*

Physica Status Solidi (A), 215(12), p.1800049_1 - 1800049_12, 2018/06

https://doi.org/10.1002/pssa.201800049
 被引用回数：6 パーセンタイル：30.3(Materials Science, Multidisciplinary)

Silver photodiffusion into amorphous chalcogenide has attracted much attention because of its potential applications for example in memory devices. For its development, it is important to know how Ag ions diffuse in chalcogenide layers upon light exposure. In this paper, the photo-induced effect on pre-reacted films before light exposure, originating from Ag/Ge$$_{20}$$S$$_{80}$$/Si substrate and Ge$$_{20}$$S$$_{80}$$/Ag/Si substrate is investigated, using neutron reflectivity, X-ray reflectivity, and X-ray diffraction. Two types of pre-reacted films according to the original stacking order are obtained. In both cases, a pure Ag layer almost disappeared, and there is a small amount of monoclinic Ag$$_{2}$$S. The reaction time for the photodiffusion is shorter, in both cases, than that in Ag/Ge$$_{20}$$S$$_{80}$$ with a pure Ag layer, indicating a different reaction process. After prolonged light exposure, a uniform amorphous reaction layer is produced in the films originating from the Ag/Ge$$_{20}$$S$$_{80}$$/Si substrate, while both an amorphous reaction product and the Ag$$_{2}$$S fragments exist in the films originating from Ge$$_{20}$$S$$_{80}$$/Ag/Si substrate. The mechanism of the specific photo-reaction is discussed in terms of the role of the Ag$$_{2}$$S fragments.

論文

Fano factor evaluation of diamond detectors for alpha particles

嶋岡 毅紘*; 金子 純一*; 佐藤 優樹; 坪田 雅功*; 新名 宏明*; 茶谷原 昭義*; 渡辺 幸志*; 梅沢 仁*; 杢野 由明*

Physica Status Solidi (A), 213(10), p.2629 - 2633, 2016/10

https://doi.org/10.1002/pssa.201600195
 被引用回数：10 パーセンタイル：41.22(Materials Science, Multidisciplinary)

This report is the first describing experimental evaluation of Fano factor for diamond detectors. High-quality self-standing chemical vapor deposited diamond samples were produced using lift-off method. Alpha-particle induced charge measurements were taken for three samples. A 13.1 eV $$pm$$ 0.07 eV of the average electron-hole pair creation energy and excellent energy resolution of approximately 0.3$$%$$ were found for 5.486 MeV alpha particles from an $$^{241}$$Am radioactive source. The best Fano factor for 5.486 MeV alpha particles calculated from experimentally obtained epsilon values and the detector intrinsic energy resolution was 0.382 $$pm$$ 0.007.

論文

Valence-band electronic structure evolution of graphene oxide upon thermal annealing for optoelectronics

山口 尚人*; 小川 修一*; 渡辺 大輝*; 穂積 英彬*; Gao, Y.*; 江田 剛輝*; Mattevi, C.*; 藤田 武志*; 吉越 章隆; 石塚 眞治*; et al.

Physica Status Solidi (A), 213(9), p.2380 - 2386, 2016/09

https://doi.org/10.1002/pssa.201532855
 被引用回数：13 パーセンタイル：52.49(Materials Science, Multidisciplinary)

本論文では加熱による酸化グラフェンの還元過程について報告する。酸化グラフェンにおいて酸素官能基の修飾度合いは加熱温度により制御できるため、加熱温度による価電子帯構造の変化をリアルタイム光電子分光で調べた。600$$^{circ}$$C以上の加熱により、フェルミ準位近傍の状態密度の顕著な増加が確認された。この結果は、600$$^{circ}$$Cにおいてバンドギャップが存在する酸化グラフェンからギャップが存在しない酸化グラフェンへと変化したことを示している。この成果は酸化グラフェンの光電子工学への応用を期待させるものである。

論文

Processes of silver photodiffusion into Ge-chalcogenide probed by neutron reflectivity technique

坂口 佳史*; 朝岡 秀人; 魚住 雄輝; 川北 至信; 伊藤 崇芳*; 久保田 正人; 山崎 大; 曽山 和彦; Sheoran, G.*; Mitkova, M.*

Physica Status Solidi (A), 213(7), p.1894 - 1903, 2016/07

https://doi.org/10.1002/pssa.201533037
 被引用回数：7 パーセンタイル：34.12(Materials Science, Multidisciplinary)

アモルファスGeカルコゲナイド/銀の界面において光を照射すると拡散が促進される。非破壊かつ時間分解で観測できるJ-PARC(写楽)の中性子反射率測定を用いて、光照射によってAgが初期の急速な拡散から緩やかな拡散と2段階のプロセスを経て、界面の拡散層が形成されている様子を捉えた。

論文

New application of NV centers in CVD diamonds as a fluorescent nuclear track detector

小野田 忍; 春山 盛善; 寺地 徳之*; 磯谷 順一*; 加田 渉*; 花泉 修*; 大島 武

Physica Status Solidi (A), 212(11), p.2641 - 2644, 2015/11

https://doi.org/10.1002/pssa.201532219
 被引用回数：11 パーセンタイル：44.98(Materials Science, Multidisciplinary)

Nitrogen-vacancy (NV) center in diamond is a luminescent point defect with applications of quantum computation and atomic scale sensors. One of the most important features of NV center is high emission rate. This enables single NV centers to be detected using a confocal laser scanning microscope. In this study, we propose a new application of NV centers as a single ion track detector. We perform 490 MeV Os ion irradiation to diamond grown by chemical vapor deposition (CVD) technique. After high temperature annealing at 1000 $$^{circ}$$C, the ion track is able to be visualized by using confocal laser scanning microscope. In short, we have successfully detected ion track in diamonds.

論文

Elemental substitution effects in multiferroic ${it R}$Fe$$_{2}$$O$$_{4}$$ (${it R}$: rare earths)

吉井 賢資; 船江 岳史*; 水牧 仁一朗*; 江尻 宏紀*; 池田 直*; 齋藤 寛之; 松村 大樹

Physica Status Solidi (C), 12(6), p.841 - 844, 2015/06

https://doi.org/10.1002/pssc.201400250
 被引用回数：1 パーセンタイル：40.68(Physics, Condensed Matter)

マルチフェロイック${it R}$Fe$$_{2}$$O$$_{4}$$ ($$R$$: Y, Ho-Lu, In)の元素置換効果について調べた。これまでほとんど報告例のない、非磁性のGa$$^{3+}$$を鉄サイトに置換した場合は、磁気転移温度$$T_{rm N}$$が減少した。これは過去、${it R}$FeCoO$$_{4}$$などでも示した通り、鉄サイト間の磁気相互作用が弱まったためである。Ga$$^{3+}$$置換した場合、室温の誘電率は母物質とほぼ変わらない1000-10000程度であった。また、誘電損失が減少することも判明した。この理由については現在不明であるが、損失の減少はエネルギー利用効率の上昇を示しており、応用に有利である。また$$R$$サイトの置換も行い、Dy$$^{3+}$$のような大きな$$R^{3+}$$を10%程置換できることが、放射光吸収分光により判明した。なお、置換試料では$$T_{rm N}$$が5-10K上昇した。この現象の起源についても現状では不明であるが、室温でマルチフェロイック状態を実現する一つの方向性を示しており、興味深い結果である。

論文

Electronic structure of BaFeO$$_{3}$$ studied by X-ray spectroscopy

水牧 仁一朗*; 藤井 将*; 吉井 賢資; 林 直顕*; 斎藤 高志*; 島川 祐一*; 魚住 孝幸*; 高野 幹夫*

Physica Status Solidi (C), 12(6), p.818 - 821, 2015/06

https://doi.org/10.1002/pssc.201400252
 被引用回数：10 パーセンタイル：94.45(Physics, Condensed Matter)

新規強磁性体BaFeO$$_{3}$$の電子状態を、放射光による高エネルギー光電子分光とX線吸収分光により調べた。実験データおよび理論計算から、この物質は負の電荷移動エネルギーを持つ系であることを示した。すなわち、酸素2p電子のエネルギーが鉄3d軌道のエネルギーより高いため、酸素2p電子が鉄3d軌道を埋めやすい性質を持っている。通常の遷移金属酸化物では、酸素2p軌道のエネルギーは遷移金属3d軌道のそれより低いため、このようなことは起こらない。すなわち、BaFeO$$_{3}$$は、通常の酸化物とは異なる性質を持つ。この性質の起源として、鉄3d軌道のクーロン反発力と、鉄3dと酸素2p軌道の強い混成であることを提案した。

論文

Shape elongation of embedded Zn nanoparticles induced by swift heavy ion irradiation; A SAXS study

雨倉 宏*; 河野 健一郎*; 大久保 成彰; 石川 法人

Physica Status Solidi (B), 252(1), p.165 - 169, 2015/01

https://doi.org/10.1002/pssb.201400138
 被引用回数：10 パーセンタイル：42.11(Physics, Condensed Matter)

Znナノ粒子に200MeV Xeイオンを照射した後、照射に伴うナノ粒子の伸長と粒子間平均距離を評価するためにSPring-8においてX線小角散乱測定を行った。高照射量領域において、小角散乱信号の方位角依存性が現れ、ナノ粒子の形状変化を検知することができた。また、イオントラック(柱状欠陥集合体)の形成に伴う小角散乱信号は、低照射量でも観測された。この結果は、イオントラックが重畳するときに新たに通過するイオントラックが事前に存在したイオントラックを消去して上書きするオーバーライティングモデルを支持するものである。また、粒子間平均距離は照射量増加に伴って増加し、小さいナノ粒子の分解と大きいナノ粒子の成長を示唆している。

論文

Optimization of substrate pretreatment and deposition conditions for epitaxial growth of $$beta$$-FeSi$$_2$$ film on Si(100)

山口 憲司; 濱本 悟*; 北條 喜一

Physica Status Solidi (C), 10(12), p.1699 - 1703, 2013/12

https://doi.org/10.1002/pssc.201300355
 被引用回数：0 パーセンタイル：0.01(Nanoscience & Nanotechnology)

シリサイド系半導体の代表格である$$beta$$-FeSi$$_2$$に対して、筆者らはスパッタ洗浄による基板前処理を併用したイオンビームスパッタ蒸着法によって、高配向した$$beta$$-FeSi$$_2$$薄膜の作製に成功している。しかし、最近、成膜温度によって高配向膜が得られる基板前処理条件が異なることがわかった。このことは、基板処理後加熱アニールを行っているとはいえ、スパッタ中に導入された照射欠陥が、少量ながらもシリサイド生成反応に影響を与えていることを示している。本研究では、$$beta$$-FeSi$$_2$$薄膜の配向性に対するスパッタ洗浄時のNe$$^+$$イオンフルエンスに対する依存性を詳細に調べ、薄膜の成長過程における照射欠陥の役割を検討した。

論文

RBS study of disordering of Fe$$_{3-x}$$Mn$$_{x}$$Si/Ge(111) heteroepitaxial interfaces

野口 雄也*; 平田 智昭*; 川久保 雄基*; 鳴海 一雅; 境 誠司; 前田 佳均

Physica Status Solidi (C), 10(12), p.1732 - 1734, 2013/12

https://doi.org/10.1002/pssc.201300380
 被引用回数：0 パーセンタイル：0.01(Nanoscience & Nanotechnology)

We have investigated thermal disordering and instability of Fe$$_{2}$$MnSi (FMS) (111)/Ge(111) heterointerfaces by Rutherford-backscattering spectrometry (RBS), and found pronounced degradation of axial orientation which appears as increase of the minimum yield of RBS when the FMS samples are annealed above 300$$^{circ}$$C. Analysis of interdiffusion at the heterointerface reveals that the disordering mainly comes from interdiffusion between Fe and Ge atoms. This situation is the same as that observed in off-stoichiometric Fe$$_{3}$$Si, ${it i.e.}$, Fe$$_{4}$$Si, but far from that in stoichiometric Fe$$_{3}$$Si.

論文

Ion beam analysis of quaternary Heusler alloy Co$$_{2}$$(Mn$$_{1-x}$$Fe$$_{x}$$)Si(111) epitaxially grown on Ge(111)

川久保 雄基*; 野口 雄也*; 平田 智昭*; 鳴海 一雅; 境 誠司; 山田 晋也*; 浜屋 宏平*; 宮尾 正信*; 前田 佳均

Physica Status Solidi (C), 10(12), p.1828 - 1831, 2013/12

https://doi.org/10.1002/pssc.201300367
 被引用回数：0 パーセンタイル：0.01(Nanoscience & Nanotechnology)

We have investigated crystal quality of Co$$_{2}$$(Mn$$_{1-x}$$Fe$$_{x}$$)Si (CMFS) epitaxially grown on Ge(111) by using Rutherford-backscattering spectrometry and an axial-ion-channeling technique. It was found that the CMFS/Ge and Co$$_{2}$$FeSi (CMFS with x = 1)/Ge have larger static atomic displacement than Fe-based ternary Heusler alloy Fe$$_{2}$$MnSi and Fe$$_{2}$$CoSi/Ge(111). Quaternary alloys may be affected by increase of mixing entropy. Significant disordering at the interface of CMFS with x = 0.75 was found, and discussed on the basis of thermodynamics.

論文

Magnetoresistance effects in current-perpendicular-to-plane structures based on Fe$$_{3}$$Si/FeSi$$_{2}$$ artificial lattices

堺 研一郎*; 野田 裕太*; 武田 薫*; 武田 全康; 吉武 剛*

Physica Status Solidi (C), 10(12), p.1862 - 1865, 2013/12

https://doi.org/10.1002/pssc.201300322
 被引用回数：1 パーセンタイル：0.01(Nanoscience & Nanotechnology)

From Fe$$_{3}$$Si/FeSi$$_{2}$$ artificial lattices, wherein FeFe$$_{3}$$Si layers are partially epitaxially grown from the first layer on Si(111) up to the top layer across the FeSi$$_{2}$$ layers with the same orientation relationship as that in the first layer, current-perpendicular-to-plane (CPP) structures that partially contain current-in-to-plane (CIP) structural portions were fabricated by a mask method. It was confirmed that the antiparallel alignment of magnetization at a zero magnetic field due to antiferromagnetic interlayer coupling is changed to parallel alignment with the applied magnetic field by polarized neutron reflectometry. The MR ratio was comparable to that of CIP structural films. It might be because a current should predominantly flow in the CIP portion since the CIP structural portion is dimensionally so large as compared with that of the CPP portion.

論文

Defect characterization in compositionally graded InGaAs layers on GaAs (001) grown by MBE

佐々木 拓生; Norman, A. G.*; Romero, M. J.*; Al-Jassim, M. M.*; 高橋 正光; 小島 信晃*; 大下 祥雄*; 山口 真史*

Physica Status Solidi (C), 10(11), p.1640 - 1643, 2013/11

https://doi.org/10.1002/pssc.201300284
 被引用回数：4 パーセンタイル：83.55(Physics, Applied)

Defect characterization in compositionally step graded In$$_{x}$$Ga$$_{1-x}$$As layers with different thickness of the overshooting (OS) layer was performed using cathodoluminescence (CL) and transmission electron microscopy (TEM). We found that the type and in-plane distribution of defects generated in the top InGaAs layer grown on step graded layers strongly depend on the thickness of the OS layer. In the thin OS layer, a high density of threading dislocations aligned along [110] was observed. In the thick OS layer, significant line defects associating composition variation were dominantly present. These features on defect type and distribution would relate to strain and configuration of the OS layer.

論文

Nonequilibrium dynamics of multiorbital correlated electron system under time-depending electric field

大西 弘明

Physica Status Solidi (B), 250(3), p.553 - 556, 2013/03

https://doi.org/10.1002/pssb.201200792
 被引用回数：0 パーセンタイル：0(Physics, Condensed Matter)

To clarify a role of orbital degrees of freedom in the response to an external field, we investigate the real-time dynamics under applied electric fields in a one-dimensional orbital degenerate Hubbard model, by exploiting numerical techniques. Let us here consider a chain along the $$z$$ axis with $$e_{rm g}$$-orbital degrees of freedom on each site and one electron per site. In the ground state, the itinerant $$d_{3z^2-r^2}$$ orbital is singly occupied and the localized $$d_{x^2-y^2}$$ orbital is empty, while the spin state exhibits antiferromagnetic correlations. After an oscillating electric field is turned on, holon-doublon pairs are created. As the time evolves, the ferro-orbital state is deformed due to the pair-hopping process that is characteristic of multi-orbital systems. Regarding the spin state, we observe the suppression of the antiferromagnetic correlations. We will also address the other filling case.

論文

Electronic states in antiferromagnet UCd$$_{11}$$ and reference compound ThCd$$_{11}$$; Studied by the de Haas-van Alphen effect

広瀬 雄介*; 三浦 泰直*; 堤 泰樹*; 吉内 伸吾*; 大家 政洋*; 杉山 清寛*; 竹内 徹也*; 山上 浩志*; 山本 悦嗣; 芳賀 芳範; et al.

Physica Status Solidi (B), 250(3), p.642 - 645, 2013/03

https://doi.org/10.1002/pssb.201200765
 被引用回数：4 パーセンタイル：20.56(Physics, Condensed Matter)

Electronic states of an antiferromagnet UCd$$_{11}$$ and its reference compound ThCd$$_{11}$$ were investigated by means of de Haas-van Alphen (dHvA) effect. From the cyclotron effective mass determined from the dHvA oscillation, the electronic specific heat of UCd$$_{11}$$ was estimated as 100 mJ/K$$^2$$mol, much smaller than 840 in the previous report. The result suggests that magnetic excitation contributes significantly to the specific heat.

論文

Gutzwiller method for heavy-fermion systems under a magnetic field

久保 勝規

Physica Status Solidi (C), 10(3), p.544 - 548, 2013/03

https://doi.org/10.1002/pssc.201200762
 被引用回数：5 パーセンタイル：89.82(Materials Science, Multidisciplinary)

We study the periodic Anderson model under a magnetic field by the Gutzwiller method. In this study, we set the Coulomb interaction between $$f$$ electrons infinity, and we consider the variational wave function given by $$| psi rangle =P | phi_{uparrow} rangle otimes | phi_{downarrow} rangle,$$ where $$P=prod_{i}[1-n_{f i uparrow}n_{f i downarrow}]$$ excludes the double occupancy of $$f$$ electrons at the same site and $$n_{f i sigma}$$ is the number operator of the $$f$$ electron with spin $$sigma$$ at site $$i$$. $$| phi_{sigma} rangle$$ denotes the one-electron part of the wave function. We evaluate energy of the variational wave function by using Gutzwiller approximation, and determine the variational parameters in the one-electron part which minimize energy. Then, spin-dependent effective mass and magnetization under a magnetic field are obtained.

論文

Measurement of oxygen chemical diffusion in PuO$$_{2-x}$$ and analysis of oxygen diffusion in PuO$$_{2-x}$$ and (Pu,U)O$$_{2-x}$$

加藤 正人; 内田 哲平; 砂押 剛雄*

Physica Status Solidi (C), 10(2), p.189 - 192, 2013/02

https://doi.org/10.1002/pssc.201200454
 被引用回数：5 パーセンタイル：89.82(Materials Science, Multidisciplinary)

It is well known that PuO$$_{2}$$ having fluorite structure is non-stoichimetric compound. Stoichiometry significantly affects physical properties such as lattice parameter, diffusion coefficient and thermal conductivity. In previous work, oxygen potential of PuO$$_{2-x}$$ was determined as functions of O/M ratio and temperature, and the data was analyzed based on defect chemistry. This result shows that the defect cluster of oxygen vacancy is stable in non-stoichiometric PuO$$_{2}$$. In this work, chemical diffusion of the defect was investigated in PuO$$_{2-x}$$. The thermo gravimeter was employed for the measurement. The O/M ratio was estimated from the weight change of the specimen. The time dependence of O/M change was analyzed, and chemical diffusion coefficient was determined as a function of temperature. The measured data was compared with that of MOX which was reported in previous work. The diffusion coefficient decreased with Pu content.

論文

Effect of oxygen-to-metal ratio on densification behavior in the sintering process of PuO$$_{2}$$ pellet

内田 哲平; 砂押 剛雄*; 加藤 正人

Physica Status Solidi (C), 10(2), p.193 - 196, 2013/02

https://doi.org/10.1002/pssc.201200475
 被引用回数：4 パーセンタイル：86.32(Materials Science, Multidisciplinary)

MOX fuel pellets are produced from UO$$_{2}$$ and PuO$$_{2}$$ powders by mechanical blending method. It is important to control pellet density in the pellet production. To investigate the change of the sintering rate depending on O/M ratio is important for MOX pellet production. The purpose of this work is to investigate the densification behavior of PuO$$_{2}$$ which is one of the starting materials as a function of O/M ratio. Thermal dilatometer was employed to measure pellet densification. The measurements were carried out in atmosphere of air and Ar/H$$_{2}$$ gas mixture added moisture. Powder of PuO$$_{2}$$ was pressed and measured at 1923 K in various conditions. The changes of grain size and densification rate were observed with O/M ratio. The PuO$$_{2}$$ pellet sintered in air was very low density of 84%TD. The highest density pellet of 96%TD was obtained by sintering at O/M ratio of about 1.99.

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